My advise would be to pick the brain box first, because that selection will drive a lot of your other selections. If you are computer savvy, I'd suggest a Megasquirt system, because they are fairly inexpensive and well sorted out. I've also used the FAST system with good results, although it was pretty expensive. My ems-pro system worked, but gave me starting problems in some cases. Both of my Mustangs are now running the Megasquirt MS3X system, and the Galaxie uses the FAST system.
You will typically need an electronic ignition setup to use with the EFI box, either a crank trigger setup or a distributor with a "crank" sensor, and maybe a cam sensor if you want to go full sequential injection with the EFI. You will also need an Air Temperature Sensor (ATS), Coolant Temperature Sensor (CTS), Throttle Position Sensor (TPS), and a Manifold Absolute Pressure sensor (MAP). And of course the wideband O2 sensors for tuning. Your fuel pump needs to be able to deliver the fuel at 45 psi or higher. The idle air control motor is optional, and I have never used one; I just use a normal hard throttle stop.
I think rather than just buying the throttle butterflies you might be better off buying a carb base plate, and machining a top to fit. Then you don't have to worry about the fit of the butterflies to your throttle body.
Last comment is once you go EFI, you'll never go back. The tunability is unbelievable.